Reaction Chemistry of W-Mn/SiO2 Catalyst for the Oxidative Coupling of Methane Reaction Chemistry of W-Mn/SiO2 Catalyst for the Oxidative Coupling of Methane

Reaction Chemistry of W-Mn/SiO2 Catalyst for the Oxidative Coupling of Methane

  • 期刊名字:天然气化学
  • 文件大小:
  • 论文作者:Shuben Li
  • 作者单位:State Key Laboratory for Oxo Synthesis and Selective Oxidation
  • 更新时间:2022-12-12
  • 下载次数:
论文简介

Reaction chemistry of the OCM reaction on W-Mn/SiO2 catalyst has been reviewed in thisaccount. Initial activity and selectivity, stability in a long-term reaction, reaction at elevated pressures anda modelling test in a stainless-steel fluidized-bed reactor show that W-Mn/SiO2 has promising performancefor the development of an OCM process that directly produces ethylene from natural gas. A study onsurface catalytic reaction kinetics and used catalyst structure characterization revealed a possible reasonwhy C2 and COx selectivity changed during the long-term reaction. Further improvement of the catalystcomposition and preparation method should be a future direction of study on OCM reaction over W-Mn/SiO2 catalyst.

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